Hostname: page-component-54dcc4c588-ff9ft Total loading time: 0 Render date: 2025-10-10T20:34:19.967Z Has data issue: false hasContentIssue false

Experimental Study of Gas Permeabilities and BreakthroughPressures in Clays

Published online by Cambridge University Press:  03 September 2012

K. Tanai
Affiliation:
Geological Isolation Technology Section, PNC Tokai Works, Tokai-mura, Ibaraki, JAPAN.
T. Kanno
Affiliation:
Geological Isolation Technology Section, PNC Tokai Works, Tokai-mura, Ibaraki, JAPAN.
C. Gallé
Affiliation:
Département d'Entreposage et de Stockage des Déchets, CEA Saclay, 91191 Gif-sur-yvette, FRANCE.
Get access

Abstract

In this study, gas migration experiments in unsaturated and saturated stateswere carried out to clarify the fundamental gas migration characteristics incompacted bentonite to be used for the geological disposal of high-levelradioactive waste. In unsaturated experiments, the gas permeability forJapanese bentonite (Kunigel VI) as a function of degree of saturation wasmeasured to examine the applicability of conventional two-phase flow modelsto compacted bentonite. The intrinsic permeability obtained in this studywas about five orders of magnitude larger than that obtained in waterpermeation tests with the same density. The difference seems to originatefrom the change of pore structure due to the swelling phenomenon of thebentonite. Since these effects have not been evaluated quantitatively yet,various relative gas permeability functions of conventional two-phase flowmodels were applied as a first approximation.

Saturated experiments designed to simulate the gas migration phenomenon in arepository for the waste were carried out to obtain relationship betweenbreakthrough and swelling pressures using Kunigel VI and French Fo-Ca clayin saturation state. The reproducibility of the breakthrough pressure wasalso examined for Kunigel VI bentonite. The breakthrough pressure was almostthe same as swelling pressure irrespective of the type of clay. As to thereproducibility of breakthrough pressure, it was observed that first andsecond breakthrough pressures were almost the same for Kunigel VI specimenswith the dry densities of 1.7 and 1.8 g/cm3.

Information

Type
Research Article
Copyright
Copyright © Materials Research Society 1997

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

Article purchase

Temporarily unavailable

References

REFERENCES

[1] PNC, Research and development on geological disposal of high level radioactive waste, First progress report, PNC TNI 410 93–059, 1992.Google Scholar
[2] Handbook of Petroleum Industry (Society of Japan petroleum Engineers, 1983, in Japanese).Google Scholar
[3] Kanno, T., Takeuchi, S. and Suzuki, H., Temperature dependence of hydraulic conductivity of compacted bentonite, PNC TN 1100 94–003, 1994.Google Scholar
[4] Michaux, L. and Loubignac, J.M., Etude microstructurale du matériau Fo-Ca, Evolution de la microstructure de l'argile Fo-Ca 7 compactée lors d'un cycle d'hydration/dehydration à 25 °C, CEA NT-SESD/95.37, 1995.Google Scholar
[5] Corey, A.T., Mechanics of immiscible fluids in porous media, Water resources publications, Littleton, Colorado, 1986.Google Scholar
[6] Fatt, I. and Klikoff, W.A., Effect of fractional wattability on multiphase flow through porous media, AEA Transactions, vol. 216, p. 246, 1959.Google Scholar
[7] Webb, S.W., Sensitivity studies for gas release from the waste isolation pilot plant (WIPP), Proceeding of OECD/NEA workshop, pp. 309326, Paris, 1992.Google Scholar
[8] Takeuchi, S. and Hara, K., Two-phase water movement in buffer material for geological isolation of high-level radioactive waste, PNC TN 8410 93–302. 1994, (in Japanese).Google Scholar
[9] Gallé, C. and Tanai, K., Gas transport in engineered barrier for nuclear waste disposal “H2 migration experiments in Fo-Ca clay”, 1996.Google Scholar
[10] Pusch, R., Ranhagen, L. and Nillson, K., Gas migration through MX-80 bentonite, Nagra TR 85–36, 1985.Google Scholar